was going to mention Pelekas, take a walk up to the Kaisers lookout and see the wonderfull views over the island.
Dont know how your budget is but we used to take an overnight bag with us, take our time going south, all the small roads and see some realy quaint places.If we found a place that was special we would take a room for the night.Just ask in a taverna if you dont see any signes, there is sure to be a room available.Take a look first, then agree on a price.dont be affraid to say no if its too much.By staying over for a night your not covering the same ground each day.Would say the west coast is the best, once your on the west side you hit the big coast road, not as nice to drive.